Two vdevs of two drives would normally be two mirrors striped together. This is often known as RAID10, although ZFS calls it "striped mirrors".
Some obligatory warnings:
It is not possible to add a drive to a RAIDZ1 to make it a RAIDZ2. After the vdev is created, the only way to change it is to back up the data elsewhere, destroy the volume, and then create the new one.
RAIDZ1 is not recommended for large drives like this. The problem is that it takes a long time to resilver big drives, and the odds of a second drive failing while the first is being replaced are too high. And if two out of three drives fail in a RAIDZ1, the volume is lost. The size limit for RAIDZ1 should be three 4TB drives. Many here in the forums recommend no more than three 1TB drives in RAIDZ1. Some also say that LZ4 compression changes those numbers, but it only means that the size limit is fuzzy, it's still there. RAIDZ2 gives two drives of redundancy, so even if a second drive fails while the first is being replaced, the pool is still working and data is not lost.