Just finished this morning (finished some time in the middle of the night) and it did indeed mount this time. The drive is resilvering so when it finishes, I'll pull the other drive and wipe it using DBAN.
Something I can now confirm is that the RAID card did indeed limit the partition size, which is why I could never get the drive to grow. I know this because the first time I attempted to wipe the drive, I stuck it into my Windows desktop and used disk manager to delete the partition. Before deleting the partition, I noted that the partitioned size was 2.2TB (exactly what FreeNAS was seeing), and it had 1.8TB of unallocated space. So it seem that once the drive was partitioned, FreeNAS couldn't grow it (which is reasonable).
Once everything is finished, I'll report back.