Hi Majerus,
There are many different ways of doing encryption... One is indeed to do it at the pool level using ZFS logical features. This can not be used for dataset because datasets are dynamic. They can be resized, increased, decreased, etc. Also, because ZFS is copy-on-write, doing such a kind of dataset-level encryption would not be easy, if even possible.
Still, you can encrypt using other features.
One option would be to create a dataset as a zvol and export it to another operating system like Linux. Linux will then be able to format it the way you wish, like an encrypted LVM. That would ensure everything in that dataset will be encrypted. It will just not be encrypted by ZFS or FreeNAS.
You can also create a share and mount it from another computer. On that one, you can use an encryption tool like Veracrypt to create a large file that will be mounted as a volume. That logical volume created by Veracrypt will also be encrypted.
So ZFS by itself will not encrypt a dataset, but there are options for you to do it or do something similar.
Always be careful with encryption and don't shoot yourself in the foot. Ensure you can do key recovery, backup and restore, etc, so encryption does not end up a tool that prevent you accessing your own data.